功能化离子液体活性位点强化CO<sub>2</sub>捕集

张威; 张瑞娜; 葛春亮; 李来; 范雯阳; 卢晗锋; 陈瑶姬; 崔国凯

doi:10.12434/j.issn.2097-2547.20240183

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功能化离子液体活性位点强化CO₂捕集

二氧化碳捕集

- 功能化离子液体活性位点强化CO₂捕集
- Intensification of CO₂ capture by active sites in functional ionic liquids
- 低碳化学与化工 2024, 49(7): 23-33.
- 作者机构：
  
  1.浙江浙能科技环保集团股份有限公司,浙江杭州 310012
  2.浙江工业大学化学工程学院催化反应工程研究所,浙江杭州 310014
- 作者简介：
  
  张威（1989—），硕士，工程师，研究方向为能源环境工程，E-mail：zhangwei9@zjenergy.com.cn。
  崔国凯（1984—），博士，研究员，研究方向为离子液体碳捕集与利用，E-mail：chemcgk@163.com。
- 基金信息：
  
  国家自然科学基金(22078294;22378353);浙江省重点研发项目(2024C03108;2023C03127);浙江浙能科技环保集团股份有限公司项目(ZNKJ-2024-077)
- DOI：10.12434/j.issn.2097-2547.20240183
  中图分类号： TQ534.9
- 纸质出版日期：2024-07-25，
  
  收稿日期：2024-04-27，
  
  修回日期：2024-05-27，
- 稿件说明：
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张威,张瑞娜,葛春亮等.功能化离子液体活性位点强化CO₂捕集[J].低碳化学与化工,2024,49(07):23-33.

ZHANG Wei,ZHANG Ruina,GE Chunliang,et al.Intensification of CO₂ capture by active sites in functional ionic liquids[J].Low-carbon Chemistry and Chemical Engineering,2024,49(07):23-33.
张威,张瑞娜,葛春亮等.功能化离子液体活性位点强化CO₂捕集[J].低碳化学与化工,2024,49(07):23-33. DOI： 10.12434/j.issn.2097-2547.20240183.

ZHANG Wei,ZHANG Ruina,GE Chunliang,et al.Intensification of CO₂ capture by active sites in functional ionic liquids[J].Low-carbon Chemistry and Chemical Engineering,2024,49(07):23-33. DOI： 10.12434/j.issn.2097-2547.20240183.

摘要

碳捕集、利用与封存（CCUS）技术已经成为我国碳中和技术体系的重要组成部分。与工业领域常用的有机胺吸收剂相比，具有低挥发性、高稳定性和位点可设计等优点的功能化离子液体在化学吸收法捕集CO

方面表现出独特的优势。综述了近年来功能化离子液体在CO

捕集领域的研究进展，简述了功能化离子液体的结构分类和合成策略，详细阐述了功能化离子液体与CO

发生化学反应的3类活性位点（氮位点、氧位点和碳位点）及相应捕集机理，并对将来功能化离子液体CO

捕集技术的研究方向进行了展望。

Abstract

Carbon capture

utilization and storage (CCUS) technology has become an important part of China’s carbon neutral technologies. Compared with the organic amine absorbers conventionally used in the industrial field

functional ionic liquids with low volatility

high stability and site designability show unique advantages in CO

capture by chemical absorptions. The research progress of functional ionic liquids for CO

capture in recent years was reviewed. The structural classification and synthesis strategies of functional ionic liquids were briefly described. Three types of active sites (nitrogen site

oxygen site and carbon site) of functional ionic liquids and the corresponding capture mechanisms were described in detail. And the future research directions of CO

capture by functional ionic liquids were prospected.

关键词

功能化离子液体CO2捕集活性位点

Keywords

functional ionic liquidsCO2 captureactive sites

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功能化离子液体活性位点强化CO2捕集

Intensification of CO2 capture by active sites in functional ionic liquids

DOI：10.12434/j.issn.2097-2547.20240183

摘要

Abstract

关键词

Keywords

references

功能化离子液体活性位点强化CO₂捕集

Intensification of CO₂ capture by active sites in functional ionic liquids