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烟道气CO2捕集用醇胺溶液降解研究进展
Research progress on degradation of alcoholamine solution for CO2 capture in flue gas
- 低碳化学与化工 2024, 49(7): 13-22.
- 作者机构：
1.中国矿业大学 碳中和研究院，江苏 徐州 221116
2.中国矿业大学 化工学院，江苏 徐州 221116
- 作者简介：
陆诗建（1984—），博士，研究员，博士研究生导师，研究方向为CCUS与废气治理技术，E-mail：lushijian@cumt.edu.cn。
- 基金信息：政府间国际科技创新合作项目(2022YFE0115800);江苏省科技厅科技项目(BE2022613);江苏省煤基温室气体减排与资源化利用重点实验室创新能力建设专项(2020ZDZZ01A)
DOI：10.12434/j.issn.2097-2547.20230347
中图分类号： TQ413纸质出版日期：2024-07-25，
收稿日期：2023-10-19，
修回日期：2023-12-20，
- 稿件说明：
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陆诗建,王风,刘玲等.烟道气CO2捕集用醇胺溶液降解研究进展[J].低碳化学与化工,2024,49(07):13-22.
LU Shijian,WANG Feng,LIU Ling,et al.Research progress on degradation of alcoholamine solution for CO2 capture in flue gas[J].Low-carbon Chemistry and Chemical Engineering,2024,49(07):13-22.
陆诗建,王风,刘玲等.烟道气CO2捕集用醇胺溶液降解研究进展[J].低碳化学与化工,2024,49(07):13-22. DOI： 10.12434/j.issn.2097-2547.20230347.
LU Shijian,WANG Feng,LIU Ling,et al.Research progress on degradation of alcoholamine solution for CO2 capture in flue gas[J].Low-carbon Chemistry and Chemical Engineering,2024,49(07):13-22. DOI： 10.12434/j.issn.2097-2547.20230347.
摘要
目前在多种CO
2
吸收捕集技术中，醇胺法是吸收量最大、经济效益最好和研究最广泛的方法。然而，醇胺法中使用的醇胺溶液吸收剂面临的降解问题是该方法的主要缺陷。针对醇胺溶液吸收剂的降解问题，首先综述了热降解和氧化降解的产物、机理和控制研究进展，然后综述了金属离子催化降解的降解机理、规律和控制研究进展，最后对醇胺溶液吸收剂的降解问题进行了总结，并对未来的抗降解研究方向进行了展望。
Abstract
At present
among the various CO
2
absorption and capture technologies
the alcoholamine method is the most widely studied method with the largest amount of absorption and the best economic benefit. However
the degradation of the alcoholamine solution absorbents used in the alcoholamine method is the main defect. In view of the problem of the degradation of alcoholamine solution absorbents
the research progress on products
mechanisms and controls of thermal degradation and oxidative degradation were first reviewed. And then the research progress on mechanisms
rules and controls of metal ion catalytic degradation were reviewed. Finally
the degradation problem of alcoholamine solution absorbents was summarized
and the future research direction of anti-degradation was prospected.
关键词
CO2捕集热降解氧化降解金属离子催化降解抗降解
Keywords
CO2 capturethermal degradationoxidative degradationmetal ion catalytic degradationanti-degradation
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