二氧化碳捕集用吸附分离技术及其吸附材料研究进展

陈久弘; 王毅; 王恺华; 陈杨; 杨江峰; 李晋平; 李立博

doi:10.12434/j.issn.2097-2547.20230261

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二氧化碳捕集用吸附分离技术及其吸附材料研究进展

二氧化碳捕集与利用

- 二氧化碳捕集用吸附分离技术及其吸附材料研究进展
- Research progress on adsorption and separation technologies and adsorption materials for carbon dioxide capture
- 低碳化学与化工 2023, 48(5): 62-70.
- 作者机构：
  
  1.太原理工大学化学工程与技术学院，山西太原 030024
- 作者简介：
  
  陈久弘（1999—），硕士研究生，研究方向为CO2捕集，E-mail：1136474391@qq.com。
  陈杨（1988—），博士，副研究员，硕士生导师，研究方向为多孔材料制备与气体吸附分离，E-mail：chenyangtyut@163.com。
- 基金信息：
  
  山西省基础研究计划(202203021223004;202203021224005);国家自然科学基金(22278288)
- DOI：10.12434/j.issn.2097-2547.20230261
  中图分类号：
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陈久弘, 王毅, 王恺华, 等. 二氧化碳捕集用吸附分离技术及其吸附材料研究进展[J]. 低碳化学与化工, 2023,48(5):62-70.

CHEN Jiuhong, WANG Yi, WANG Kaihua, et al. Research progress on adsorption and separation technologies and adsorption materials for carbon dioxide capture[J]. Low-carbon Chemistry and Chemical Engineering, 2023,48(5):62-70.
陈久弘, 王毅, 王恺华, 等. 二氧化碳捕集用吸附分离技术及其吸附材料研究进展[J]. 低碳化学与化工, 2023,48(5):62-70. DOI： 10.12434/j.issn.2097-2547.20230261.

CHEN Jiuhong, WANG Yi, WANG Kaihua, et al. Research progress on adsorption and separation technologies and adsorption materials for carbon dioxide capture[J]. Low-carbon Chemistry and Chemical Engineering, 2023,48(5):62-70. DOI： 10.12434/j.issn.2097-2547.20230261.

摘要

为缓解温室效应带来的一系列严重的环境问题，亟需对主要的温室气体二氧化碳（CO,2,）进行减排。CO,2,的捕集、利用与封存（CCUS）技术作为可以有效进行碳减排，得到了广泛应用。在CO,2,捕集技术中，物理吸附分离技术具有能耗低、产品气质量稳定和适应性强等优点，可推广至不同工业应用场景。介绍了3种吸附分离技术的CO,2,捕集场景：燃烧后烟气捕集、天然气净化以及直接空气捕集，以及可用于吸附分离技术的4种CO,2,吸附材料：多孔碳材料、沸石分子筛、硅基材料与金属有机骨架材料，并对以上材料的适用条件与场景进行了总结，最后对CO,2,吸附剂未来的发展方向进行了展望。

Abstract

In order to alleviate a series of serious environmental problems caused by greenhouse effect, it is urgent to reduce the main greenhouse gas, carbon dioxide (CO,2,) emissions. CO,2, capture, utilization and storage (CCUS) technology has been widely used as an effective method to reduce carbon emissions. Among CO,2, capture technologies, physical adsorption separation technology has the advantages of low energy consumption, stable product gas quality and strong adaptability, and can be extended to different industrial application scenarios. Three CO,2, capture scenarios for adsorption and separation technologies: post-combustion flue gas capture, natural gas purification and direct air capture, and four kinds of CO,2, adsorbent materials: porous carbon materials, zeolite molecular sieves, silicon-based materials and metal-organic framework materials were introduced. The applicable conditions and scenarios of the above materials were summarized, and the future development direction of CO,2, adsorbents was prospected.

关键词

CO2捕集多孔材料物理吸附变压吸附

Keywords

CO2 captureporous materialphysical adsorptionpressure swing adsorption

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