燃烧后二氧化碳捕集材料的研究进展

于小荣; 吉仁静; 杨欢; 王尔珍; 苏高申

doi:10.12434/j.issn.2097-2547.20230124

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燃烧后二氧化碳捕集材料的研究进展

二氧化碳捕集与利用

- 燃烧后二氧化碳捕集材料的研究进展
- Research progress of post-combustion carbon dioxide capture materials
- 低碳化学与化工 2023, 48(5): 82-94.
- 作者机构：
  
  1.长江大学化学与环境工程学院，湖北荆州 434100
  2.长庆油田油气工艺研究院，陕西西安 710018
- 作者简介：
  
  于小荣（1988—），博士，讲师，研究方向为油气田应用化学，E-mail：yxr_cjdx@163.com。
  杨欢（1981—），博士，副教授，研究方向为油气田应用化学，E-mail：yanghuan@yangtzeu.edu.cn；
- 基金信息：
  
  国家自然科学基金企业创新发展联合基金(U19B6003-05)
- DOI：10.12434/j.issn.2097-2547.20230124
  中图分类号：
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于小荣, 吉仁静, 杨欢, 等. 燃烧后二氧化碳捕集材料的研究进展[J]. 低碳化学与化工, 2023,48(5):82-94.

YU Xiaorong, JI Renjing, YANG Huan, et al. Research progress of post-combustion carbon dioxide capture materials[J]. Low-carbon Chemistry and Chemical Engineering, 2023,48(5):82-94.
于小荣, 吉仁静, 杨欢, 等. 燃烧后二氧化碳捕集材料的研究进展[J]. 低碳化学与化工, 2023,48(5):82-94. DOI： 10.12434/j.issn.2097-2547.20230124.

YU Xiaorong, JI Renjing, YANG Huan, et al. Research progress of post-combustion carbon dioxide capture materials[J]. Low-carbon Chemistry and Chemical Engineering, 2023,48(5):82-94. DOI： 10.12434/j.issn.2097-2547.20230124.

摘要

二氧化碳（CO,2,）的过量排放造成了气候变化、生态失衡和海洋酸化等一系列严重问题，CO,2,捕集与封存（CCS）技术是目前能缓解CO,2,过量排放的有效手段。在CCS技术中，CO,2,捕集环节所需的成本最高，为了使CCS技术得到有效推广和应用，应重点研究CO,2,捕集技术和材料以降低该环节的成本。在3种CO,2,捕集技术中，与燃烧前捕集技术和富氧燃烧技术相比，燃烧后捕集技术因技术成熟、对设备改造要求低而被广泛应用。重点综述了燃烧后CO,2,捕集材料的研究进展，包括液体吸收剂（有机胺、氨水溶液和离子液体）、固体吸附剂（生物炭、沸石和金属有机框架材料等）以及膜材料，并对比分析了各种材料的优缺点。最后提出干水因其独特的“固包液”结构可作为一种固液复合CO,2,捕集材料，有望克服单一材料的缺点，提高CO,2,捕集效率。

Abstract

The excessive emission of carbon dioxide (CO,2,) has caused a series of serious problems such as climate change, ecological unbalance, ocean acidification and so on. CO,2, capture and storage (CCS) technology is an effective means to alleviate the excessive emission of CO,2, at present. Among CCS technologies, CO,2, capture requires the highest cost. In order to effectively promote and apply CCS technology, emphasis should be placed on CO,2, capture technology and materials to reduce the cost of this process. Among the three CO,2, capture technologies, compared with pre-combustion capture technology and oxy-combustion technology, post-combustion capture technology has been widely used because of its mature technology and low requirements for equipment transformation. The research progress of CO,2, capture materials after combustion was reviewed, including liquid absorbent (organic amine, ammonia solution and ionic liquid), solid adsorbent (biochar, zeolite, metal-organic frame materials, etc.) and membrane materials, and advantages and disadvantages of each materials were compared and analyzed. Finally, it was proposed that dry water can be used as a solid-liquid composite CO,2, capture material because of its unique “solid-liquid” structure, which is expected to overcome the shortcomings of a single material and improve the CO,2 ,capture efficiency.

关键词

CO2捕集液体吸收剂固体吸附剂膜分离干水

Keywords

CO2 captureliquid absorbentsolid adsorbentmembrane separationdry water

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