Research progress in preparation of fly ash based aluminosilicate materials and their CO<sub>2</sub> capture

PANG Wei; QIN Shenjun; HAO Longlong; MEN Changquan; HOU Jiajia; LI Shenyong

doi:10.12434/j.issn.2097-2547.20240010

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Research progress in preparation of fly ash based aluminosilicate materials and their CO₂ capture

- Research progress in preparation of fly ash based aluminosilicate materials and their CO₂ capture
- Vol. 49, Issue 7, Pages: 42-54(2024)
- 作者机构：
  
  1.河北工程大学材料科学与工程学院，河北邯郸 056038
  2.河北工程大学河北省资源勘测研究重点实验室，河北邯郸 056038
- 作者简介：
- 基金信息：
- DOI：10.12434/j.issn.2097-2547.20240010
  CLC： TQ536.4
- Published：25 July 2024，
  
  Received：06 January 2024，
  
  Revised：01 March 2024，
- 稿件说明：
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庞薇,秦身钧,郝龙龙等.粉煤灰基硅铝酸盐材料的合成及其捕集CO₂的研究进展[J].低碳化学与化工,2024,49(07):42-54.

PANG Wei,QIN Shenjun,HAO Longlong,et al.Research progress in preparation of fly ash based aluminosilicate materials and their CO₂ capture[J].Low-carbon Chemistry and Chemical Engineering,2024,49(07):42-54.
庞薇,秦身钧,郝龙龙等.粉煤灰基硅铝酸盐材料的合成及其捕集CO₂的研究进展[J].低碳化学与化工,2024,49(07):42-54. DOI： 10.12434/j.issn.2097-2547.20240010.

PANG Wei,QIN Shenjun,HAO Longlong,et al.Research progress in preparation of fly ash based aluminosilicate materials and their CO₂ capture[J].Low-carbon Chemistry and Chemical Engineering,2024,49(07):42-54. DOI： 10.12434/j.issn.2097-2547.20240010.

摘要

大量排放导致全球变暖加剧，碳捕集可减缓CO

排放对气候变化的影响，但吸附剂高昂的成本阻碍了碳捕集技术的发展。同时煤炭燃烧量持续增加使粉煤灰产量不断增加，而粉煤灰的高值化利用率较低。将

粉煤灰用于合成粉煤灰基硅铝酸盐材料，并应用于碳捕集技术可实现工业固体废物的高值化利用和碳减排的双重目标。介绍了粉煤灰合成硅铝酸盐材料前的预处理步骤，系统讨论了粉煤灰基沸石、Li

SiO

吸附剂和SiO

介孔材料的合成和其捕集CO

的研究，然后对粉煤灰基硅铝酸盐材料吸附CO

的动力学进行了总结。粉煤灰基硅铝酸盐材料制备前的物理和化学预处理步骤可优化材料的孔隙结构及表面化学性质，胺功能化或金属离子掺杂等方式可实现对材料结构和CO

吸附性能的调控。粉煤灰基硅铝酸盐材料的CO

吸附动力学拟合因产物及吸附条件不同而存在差异。深入理论研究，推动规模化工程应用，对促进碳捕集技术发展具有重要的指导意义。

Abstract

The escalating emissions of CO

exacerbate global warming. Carbon capture offers a potential avenue to attenuate CO

emissions

but the high cost of adsorbents acts as a barrier to the development of carbon capture technologies. Simultaneously

the continual increase in coal combustion leads to a rise in fly ash production

yet its valorization remains relatively low. Utilizing fly ash for synthesizing fly ash-based aluminosilicate materials and their application in carbon capture technologies present a dual solution by valorizing industrial solid waste and reducing carbon emissions. The preprocessing steps prior to synthesizing fly ash-based aluminosilicate materials were outlined and the research on synthesis of fly ash-based zeolites

SiO

adsorbents

and SiO

mesoporous materials and their synthesis were systematically discussed

and the kinetics of CO

adsorption on fly ash-based aluminosilicate materials were summarized. Physical and chemical preprocessing steps before preparing fly ash-based aluminosilicate materials optimize the materials’ pore structure and surface chemical properties. Strategies such as amine functionalization or metal ion doping enable control over the material structure and CO

capture performance. Discrepancies in the kinetics of CO

capture on fly ash-based aluminosilicate materials arise from variations in reaction products and capture conditions. In-depth theoretical research and promoting large-scale engineering applications hold significant promise

in guiding the development of carbon capture technologies.

关键词

粉煤灰CO2捕集硅铝酸盐材料吸附动力学

Keywords

fly ashCO2 capturealuminosilicate materialsadsorption kinetics

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Research progress in preparation of fly ash based aluminosilicate materials and their CO2 capture

DOI：10.12434/j.issn.2097-2547.20240010

摘要

Abstract

关键词

Keywords

references

Research progress in preparation of fly ash based aluminosilicate materials and their CO₂ capture