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煤/煤焦与天然气协同转化研究进展
Research progress on synergistic conversion of coal/coal char and natural gas
- 低碳化学与化工 2025, 50(8): 1-11.
- 作者机构：
1.西北大学 化工学院 碳氢资源清洁利用国际科技合作基地，陕北能源先进化工利用技术教育部工程研究中心，陕西省洁净煤转化工程技术研究中心，陕西 西安 710127
2.榆神工业区能源科技发展有限公司，陕西 榆林 719302
- 作者简介：
郑煜晨（2005—），本科，研究方向为煤化工与低碳化工，E-mail：2261921245@qq.com。
张建波（1986—），博士，教授，研究方向为煤与天然气化工，E-mail：jbzhang@nwu.edu.cn。
- 基金信息：陕西省青年创新团队项目(24JP182);陕西省自然科学基础研究计划-陕煤联合基金(2021JLM-22);榆林市科技计划(CXY-2022-163)
DOI：10.12434/j.issn.2097-2547.20250165
中图分类号： TQ519收稿日期：2025-04-08，
修回日期：2025-05-01，
纸质出版日期：2025-08-25
- 稿件说明：
移动端阅览
郑煜晨,王建友,窦珍等.煤/煤焦与天然气协同转化研究进展[J].低碳化学与化工,2025,50(8):1-11.
ZHENG Yuchen,WANG Jianyou,DOU Zhen,et al.Research progress on synergistic conversion of coal/coal char and natural gas[J].Low-Carbon Chemistry and Chemical Engineering,2025,50(8):1-11.
郑煜晨,王建友,窦珍等.煤/煤焦与天然气协同转化研究进展[J].低碳化学与化工,2025,50(8):1-11. DOI： 10.12434/j.issn.2097-2547.20250165.
ZHENG Yuchen,WANG Jianyou,DOU Zhen,et al.Research progress on synergistic conversion of coal/coal char and natural gas[J].Low-Carbon Chemistry and Chemical Engineering,2025,50(8):1-11. DOI： 10.12434/j.issn.2097-2547.20250165.
摘要
煤与天然气协同转化有助于两种能源资源的碳氢元素互补与节能降耗，对于发展“以煤为基多能融合”的能源体系具有重要价值和意义。我国的低阶煤资源丰富，伴随着以中低温热解为核心的煤炭分级分质利用产业的发展，大量的煤热解半焦（简称“煤焦”）亟待高值化利用，而煤焦转化通常为煤炭转化的决速步骤
在一定程度上限制了其应用路径。基于煤与天然气热转化的主要特征，简述了煤与天然气协同转化的工艺特点及相关研究，重点围绕煤炭转化的中间体——煤焦与天然气协同转化联产功能碳材料与氢气/合成气方向，从煤焦转化与甲烷裂解协同、煤焦转化与甲烷干重整协同和煤焦与中低温热解煤气协同转化三方面进行了综合评述，并展望了未来的发展方向。
Abstract
The synergistic conversion of coal and natural gas can help to achieve complementary carbon and hydrogen elements of the two energy resources and to achieve energy conservation and reduction of consumption
which has great value and significance for the development of an energy system based on coal with multi-energy integration. China is rich in low-rank coal resources
and with the development of coal classification and graded utilization industry via medium-low temperature pyrolysis
a large number of coal pyrolysis semi-coke (referred to as “coal char”) is in urgent need of high-value conversion and utilization. Especially
the conversion of coal char is usually the decisive step of coal conversion
which limits its application paths to some extent. Based on the main characteristics of thermal conversion of coal and natural gas
the process features and the related works about synergistic conversion of coal and natural gas were briefly described
focusing on the research of synergistic conversion of coal char (as an intermediate of coal conversion) and natural gas for co-production of carbon materials and hydrogen/syngas. A comprehensive review was conducted from three aspects: Integrating coal char conversion and methane cracking
integrating coal char conversion and methane dry reforming
and synergistic conversion of coal char and coal pyrolysis gas obtained at medium-low temperature. The future development direction was also prospected.
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