太阳能驱动界面蒸发中的碳基材料：碳减排机制与应用前景

李小可; 杨锐; 廖胤皓; 周立宏; 敬登伟

doi:10.12434/j.issn.2097-2547.20250066

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太阳能驱动界面蒸发中的碳基材料：碳减排机制与应用前景

分离材料与净化技术 | 更新时间：2026-02-02

- 太阳能驱动界面蒸发中的碳基材料：碳减排机制与应用前景
- Carbon-based materials in solar-driven interfacial evaporation: Carbon emission reduction mechanisms and application prospects
- 低碳化学与化工 2026, 51(1): 73-86.
- 作者机构：
  
  1.西安交通大学动力工程多相流国家重点实验室，陕西西安 710049
  2.成都理工大学材料与化学化工学院，四川成都 610059
  3.天府永兴实验室，四川成都 610213
  4.成都理工大学生态环境学院，四川成都 610059
- 作者简介：
  
  李小可（1990—），博士，副教授，研究方向为化工强化传热，E-mail：xiaokeli319@126.com。
  敬登伟（1977—），博士，教授，研究方向为能源转化系统中的微纳尺度颗粒液固两相流及其与复杂物理场、化学场的高效耦合，E-mail：dwjing@mail.xjtu.edu.cn。
- 基金信息：
  
  国家自然科学基金青年科学基金（A类）(52025061);国家自然科学基金青年科学基金（C类）(52406068);天府永兴实验室开放课题(2024KFXM08)
- DOI：10.12434/j.issn.2097-2547.20250066
  中图分类号： TK519
- 收稿：2025-02-23，
  
  修回：2025-03-06，
  
  纸质出版：2026-01-25
- 稿件说明：
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李小可,杨锐,廖胤皓等.太阳能驱动界面蒸发中的碳基材料：碳减排机制与应用前景[J].低碳化学与化工,2026,51(1):73-86.

LI Xiaoke,YANG Rui,LIAO Yinhao,et al.Carbon-based materials in solar-driven interfacial evaporation: Carbon emission reduction mechanisms and application prospects[J].Low-Carbon Chemistry and Chemical Engineering,2026,51(1):73-86.
李小可,杨锐,廖胤皓等.太阳能驱动界面蒸发中的碳基材料：碳减排机制与应用前景[J].低碳化学与化工,2026,51(1):73-86. DOI： 10.12434/j.issn.2097-2547.20250066.

LI Xiaoke,YANG Rui,LIAO Yinhao,et al.Carbon-based materials in solar-driven interfacial evaporation: Carbon emission reduction mechanisms and application prospects[J].Low-Carbon Chemistry and Chemical Engineering,2026,51(1):73-86. DOI： 10.12434/j.issn.2097-2547.20250066.

摘要

太阳能驱动界面蒸发（SIE）技术凭借其绿色环保和低能耗等优势，为应对全球水资源短缺与能源危机提供了全新解决思路。近年来，碳基材料凭借其优异的光热转换性能、大比表面积以及良好的化学稳定性，在上述领域中展现出巨大应用潜力。碳基材料能够显著提升能量转换效率，降低系统成本，同时在减少碳排放方面亦有作用。综述了碳基材料在太阳能驱动界面蒸发技术中的研究进展，重点围绕其光热转换、水传输及抗盐等机制进行深入探讨，分析其碳减排潜力，并展望其在海水淡化和污水处理等领域的应用前景，旨在为构建高效、低成本和可持续的水处理技术提供参考，以助力“碳中和”目标的实现。

Abstract

Solar-driven interfacial evaporation (SIE) technology

with its advantages of environmental friendliness and low energy consumption

offers a novel solution to the global challenges of water scarcity and energy crisis. In recent years

carbon-based materials have demonstrated great application potential in this field due to their excellent photothermal conversion performance

large specific surface area and good chemical stability. Carbon-based materials can significantly enhance energy conversion efficiency

reduce system costs

and play a role in reducing carbon emissions. The research progress of carbon-based materials in solar-driven interfacial evaporation technology was summarized

with a focus on in-depth discussion of their photothermal conversion

water transport and anti-salting mechanisms. Their potential for carbon emission reduction was analyzed

and their application prospects in seawater desalination and wastewater treatment were prospected

aming to provide a reference for the development of efficient

low-cost and sustainable water treatment technologies

contributing to the realization of “carbon neutrality” goals.

关键词

Keywords

references

ZHAO H Y , HUANG J , ZHOU J , et al . Biomimetic design of macroporous 3D truss materials for efficient interfacial solar steam generation [J ] . ACS Nano , 2022 , 16 ( 3 ): 3554 - 3562 .

GUO Y H , LU H Y , ZHAO F , et al . Biomass-derived hybrid hydrogel evaporators for cost-effective solar water purification [J ] . Advanced Materials , 2020 , 32 ( 11 ): 1907061 .

DJELLABI R , NOUREEN L , DAO V D , et al . Recent advances and challenges of emerging solar-driven steam and the contribution of photocatalytic effect [J ] . Chemical Engineering Journal , 2022 , 431 : 134024 .

BAIN R , JOHNSTON R , SLAYMAKER T . Drinking water quality and the SDGs [J ] . npj Clean Water , 2020 , 3 ( 1 ): 37 .

ELSAID K , KAMIL M , SAYED E T , et al . Environmental impact of desalination technologies: A review [J ] . Science of The Total Environment , 2020 , 748 : 141528 .

HAN X Q , ZHANG D , YAN J J , et al . Process development of flue gas desulphurization wastewater treatment in coal-fired power plants towards zero liquid discharge: Energetic, economic and environmental analyses [J ] . Journal of Cleaner Production , 2020 , 261 : 121144 .

XU S M , GUO S B , WU X , et al . Analysis of a multi-stage air gap diffusion distillation system powered by low-grade sensible heat [J ] . Applied Thermal Engineering , 2022 , 200 : 117660 .

LI Y H , CHENG S A , YU Z , et al . Stable, zero liquid discharge, and highly efficient solar-driven multistage distillation device based on tree-inspired radial water transfer [J ] . Journal of Cleaner Production , 2022 , 375 : 134025 .

WANG L , CHENG H Y , WU G , et al . Thermodynamic and economic analysis of a solar hydroponic planting system with multi-stage interfacial distillation units [J ] . Desalination , 2022 , 539 : 115970 .

GHASEMI H , NI G , MARCONNET A M . Solar steam generation by heat localization [J ] . Nature Communications , 2014 , 5 ( 1 ): 4449 .

YUAN Y , DONG C L , GU J J , et al . A scalable nickel-cellulose hybrid metamaterial with broadband light absorption for efficient solar distillation [J ] . Advanced Materials , 2020 , 32 ( 17 ): 1907975 .

LIU S , LI S T , LIN M . Understanding interfacial properties for enhanced solar evaporation devices: From geometrical to physical interfaces [J ] . ACS Energy Letters , 2023 , 8 ( 4 ): 1680 - 1687 .

DING M C , LU H , SUN Y B , et al . Superelastic 3D assembled clay/graphene aerogels for continuous solar desalination and oil/organic solvent absorption [J ] . Advanced Science , 2022 , 9 ( 36 ): 2205202 .

LI L , HE N , JIANG B . Highly salt-resistant 3D hydrogel evaporator for continuous solar desalination via localized crystallization [J ] . Advanced Functional Materials , 2021 , 31 : 2104380 .

LIU G H , CHEN T , XU J L , et al . Salt-rejecting solar interfacial evaporation [J ] . Cell Reports Physical Science , 2021 , 2 ( 1 ): 100310 .

HUANG Q Q , DU C K , HUANG C L . Nature-inspired pyramid-shaped 3-dimensional structure for cost-effective heat-localized solar evaporation with high efficiency and salt localization [J ] . Applied Thermal Engineering , 2022 , 215 : 118950 .

CHEN X , HE S M , FALINSKI M M , et al . Sustainable off-grid desalination of hypersaline waters using Janus wood evaporators [J ] . Energy & Environmental Science , 2021 , 14 ( 10 ): 5347 - 5357 .

杜恒 , 方剑 , 葛灿 , 等 . 界面光热水蒸发用碳基纤维材料的研究进展 [J ] . 复合材料学报 , 2023 , 40 ( 6 ): 3115 - 3124 .

DU H , FANG J , GE C , et al . Research progress on carbon-based fibrous materials for interfacial solar thermal water evaporation [J ] . Acta Materiae Compositae Sinica , 2023 , 40 ( 6 ): 3115 - 3124 .

杨小林 , 马立波 . 太阳能蒸汽发生装置及碳基光热转换材料研究进展 [J ] . 粉末冶金工业 , 2022 , 32 ( 4 ): 85 - 88 .

YANG X L , MA L B . Research progress on solar steam generation devices and carbon-based photothermal conversion materials [J ] . Powder Metallurgy Industry , 2022 , 32 ( 4 ): 85 - 88 .

HE W , ZHOU L , WANG M , et al . Structure development of carbon-based solar-driven water evaporation systems [J ] . Science Bulletin , 2021 , 66 ( 14 ): 1472 - 1483 .

LI Y M , SHI Y Y , WANG H W , et al . Recent advances in carbon-based materials for solar-driven interfacial photothermal conversion water evaporation: Assemblies, structures, applications, and prospective [J ] . Carbon Energy , 2023 , 5 ( 11 ): e331 .

CUI Z X , ZHOU J Q , WANG H R , et al . Facile fabrication of electrospinning cellulose acetate/graphene composite nanofiber membrane with high solar-to-thermal conversion and oil resistance performance for efficient solar-driven water evaporation [J ] . Solar Energy Materials and Solar Cells , 2023 , 263 : 112597 .

WEI W J , HE J J , HE L , et al . Study of direct drinking water production and sea salt recovery from photothermal conversion based on MWCNTs [J ] . Separation and Purification Technology , 2024 , 335 : 126068 .

WANG W , TIAN Z Y , HE N R , et al . Biomass derived evaporator with highly interconnected structure for eliminating salt accumulation in high-salinity brine [J ] . Desalination , 2024 , 574 : 117232 .

YANG R , LI X K , XIE W , et al . Exceeding the theoretical limit of interfacial evaporation efficiency by using the carbon-based aerogel evaporator with cold evaporation surface [J ] . Desalination , 2024 , 592 : 118165 .

YANG R , LI X K , YIN F , et al . The mechanism of enhanced photothermal conversion of low-dimensional plasmonic nanofluids with LFPs resonance [J ] . International Journal of Heat and Mass Transfer , 2023 , 208 : 124056 .

GAO M M , ZHU L L , PEH C K , et al . Solar absorber material and system designs for photothermal water vaporization towards clean water and energy production [J ] . Energy & Environmental Science , 2019 , 12 ( 3 ): 841 - 864 .

REN H Y , TANG M , GUAN B L , et al . Hierarchical graphene foam for efficient omnidirectional solar-thermal energy conversion [J ] . Advanced Materials , 2017 , 29 ( 38 ): 1702590 .

ZHANG P P , LI J , LV L X , et al . Vertically aligned graphene sheets membrane for highly efficient solar thermal generation of clean water [J ] . ACS Nano , 2017 , 11 ( 5 ): 5087 - 5093 .

ZHANG W B , WANG J N , WEI L F , et al . Preparation and application of functional polymer-based electromagnetic shielding materials [J ] . Progress in Chemistry , 2023 , 35 ( 7 ): 1065 - 1076 .

CUI K H , WARDLE B L . Breakdown of native oxide enables multifunctional, free-form carbon nanotube—Metal hierarchical architectures [J ] . ACS Applied Materials & Interfaces , 2019 , 11 ( 38 ): 35212 - 35220 .

ZHOU S L , ZHANG J P , WANG C , et al . Extremely black carbon nanotube materials with three-dimensional networks for highly efficient solar-driven vapor generation [J ] . Nanoscale , 2022 , 14 ( 46 ): 17438 - 17446 .

ZHAO L M , YANG Z P , WANG J J , et al . Boosting solar-powered interfacial water evaporation by architecting 3D interconnected polymetric network in CNT cellular structure [J ] . Chemical Engineering Journal , 2023 , 451 : 138676 .

DONG C S , CHEN L , LIN W Q , et al . Nature-inspired 3D hierarchical carbon nanotube matrices enable extraordinary solar steam generation [J ] . Carbon Energy , 2025 , 7 ( 3 ): e655 .

WILSON H M , AHIRRAO D J , RAHEMAN A S , et al . Biomass-derived porous carbon for excellent low intensity solar steam generation and seawater desalination [J ] . Solar Energy Materials and Solar Cells , 2020 , 215 : 110604 .

IBRAHIM I , BHOOPAL V , SEO D H , et al . Biomass-based photothermal materials for interfacial solar steam generation: A review [J ] . Materials Today Energy , 2021 , 21 : 100716 .

GAN Z C , SUN W C , ZHAO S , et al . Hierarchical porous structure salt-resistance carbon-based aerogel for efficient solar-driven interfacial steam generation [J ] . Chemical Engineering Journal , 2024 , 495 : 153694 .

GAN Z C , ZHAO S , ZHANG Z , et al . Janus structured carbon-graphene composite aerogel for high efficiency solar water evaporation [J ] . Separation and Purification Technology , 2025 , 360 : 130937 .

WU X T , LI C C , ZHANG Z Q , et al . Nitrogen-doped microporous graphite-enhanced copper plasmonic effect for solar evaporation [J ] . Carbon Energy , 2024 , 6 ( 3 ): e466 .

ZHU H W , GE J , ZHAO H Y , et al . Sponge-templating synthesis of sandwich-like reduced graphene oxide nanoplates with confined gold nanoparticles and their enhanced stability for solar evaporation [J ] . Science China Materials , 2020 , 63 ( 10 ): 1957 - 1965 .

ZHANG H , LI X K , ZHENG S Z , et al . The coral-inspired steam evaporator for efficient solar desalination via porous and thermal insulation bionic design [J ] . SmartMat , 2023 , 4 ( 6 ): e1175 .

SU X , HAO D Z , SUN M Y , et al . Nature sunflower stalk pith with zwitterionic hydrogel coating for highly efficient and sustainable solar evaporation [J ] . Advanced Functional Materials , 2022 , 32 ( 6 ): 2108135 .

BANG J W , MOON I K , OH J . Three-dimensional multimodal porous graphene-carbonized wood for highly efficient solar steam generation [J ] . Sustainable Energy Technologies and Assessments , 2023 , 57 : 103199 .

HU Y , XU J N , CHEN Y , et al . Lotus-inspired cellulose-based aerogel with Janus wettability and vertically aligned vessels for salt-rejecting solar seawater purification [J ] . Carbohydrate Polymers , 2025 , 352 : 123158 .

ABDELSALAM M A , SAJJAD M , RAZA A , et al . Sustainable biomimetic solar distillation with edge crystallization for passive salt collection and zero brine discharge [J ] . Nature Communications , 2024 , 15 ( 1 ): 874 .

WEI Y J , LI W H , ZHANG S C , et al . Laser-induced porous graphene/CuO composite for efficient interfacial solar steam generation [J ] . Advanced Functional Materials , 2024 , 34 ( 28 ): 2401149 .

HUANG D , ZHANG J , WU G , et al . A solar evaporator based on hollow polydopamine nanotubes with all-in-one synergic design for highly-efficient water purification [J ] . Journal of Materials Chemistry A , 2021 , 9 ( 28 ): 15776 - 15786 .

YANG H , SUN Y H , PENG M W , et al . Tailoring the salt transport flux of solar evaporators for a highly effective salt-resistant desalination with high productivity [J ] . ACS Nano , 2022 , 16 ( 2 ): 2511 - 2520 .

SUN B J , HAN Y , LI S W , et al . Cotton cloth supported tungsten carbide/carbon nanocomposites as a Janus film for solar driven interfacial water evaporation [J ] . Journal of Materials Chemistry A , 2021 , 9 ( 40 ): 23140 - 23148 .

HU G X , LIU H J , LIU K K , et al . All-in-one carbon foam evaporators for efficient co-generation of freshwater and electricity [J ] . Advanced Functional Materials , 2025 : 2423781 .

ZHU R F , WANG D , XIE J Y , et al . Salt-resistant Schiff base cross-linked superelastic photothermal cellulose aerogels for long-term seawater desalination [J ] . Chemical Engineering Journal , 2022 , 427 : 131618 .

ZHANG H , DU Y P , JING D W , et al . Integrated Janus evaporator with an enhanced donnan effect and thermal localization for salt-tolerant solar desalination and thermal-to-electricity generation [J ] . ACS Applied Materials & Interfaces , 2023 , 15 ( 42 ): 49892 - 49901 .

WANG W H , WANG Y , KONG X J , et al . Carbon-based material for CO 2 catalytic conversion applications [J ] . Carbon Future , 2024 , 1 ( 3 ): 9200016 .

LIU W J , JIANG H , YU H Q . Emerging applications of biochar-based materials for energy storage and conversion [J ] . Energy & Environmental Science , 2019 , 12 ( 6 ): 1751 - 1779 .

YANG X M , HE H H , LV T , et al . Fabrication of biomass-based functional carbon materials for energy conversion and storage [J ] . Materials Science and Engineering: R: Reports , 2023 , 154 : 100736 .

HU B , YU S H , WANG K , et al . Functional carbonaceous materials from hydrothermal carbonization of biomass: An effective chemical process [J ] . Dalton Transactions , 2008 , ( 40 ): 5414 - 5423 .

WU Z H , YAO C , MENG Z Z , et al . Biomass-derived crocodile skin-like porous carbon for high-performance microwave absorption [J ] . Advanced Sustainable Systems , 2022 , 6 ( 6 ): 2100454 .

KONG T C , QIAN Y , LI Y , et al . Plastic-derived sandwich-like porous carbon nanosheet-supported hexagonal carbon micro-flakes for K-ion storage [J ] . Chemical Communications , 2023 , 59 ( 28 ): 4169 - 4172 .

YU Z , GU R N , ZHANG Y X , et al . High-flux flowing interfacial water evaporation under multiple heating sources enabled by a biohybrid hydrogel [J ] . Nano Energy , 2022 , 98 : 107287 .

MAO K , ZHANG Y X , TAN S C . Functionalizing solar-driven steam generation towards water and energy sustainability [J ] . Nature Water , 2025 , 3 ( 2 ): 144 - 156 .

ZHANG Q Y , CHEN Y , WANG Y T , et al . Scalable ultralight wood-inspired aerogel with vertically aligned micrometer channels for highly efficient solar interfacial desalination [J ] . ACS Applied Materials & Interfaces , 2023 , 15 ( 43 ): 50522 - 50531 .

WANG C , ZHOU S L , WU C , et al . Janus carbon nanotube sponges for highly efficient solar-driven vapor generation [J ] . Chemical Engineering Journal , 2023 , 454 : 140501 .

HE P P , HAO L , LIU N , et al . Controllable synthesis of sea urchin-like carbon from metal-organic frameworks for advanced solar vapor generators [J ] . Chemical Engineering Journal , 2021 , 423 : 130268 .

YU S D , WEI Y J , FANG D , et al . Enhancing efficiency of interfacial solar steam generation with biomimetic hierarchical porous graphene activated by NaOH [J ] . Desalination , 2024 , 586 : 117909 .

HAN J Y , DONG Z Y , HAO L , et al . Poly(ionic liquid)-crosslinked graphene oxide/carbon nanotube membranes as efficient solar steam generators [J ] . Green Energy & Environment , 2023 , 8 ( 1 ): 151 - 162 .

HE H J , SONG X M , HUANG M N , et al . A photothermal and conductive composite hydrogel membrane for solar-driven synchronous desalination and salinity power generation [J ] . Green Chemistry , 2023 , 25 ( 22 ): 9343 - 9350 .

HUO B C , LIU S , DU C Y , et al . Organic carbonization modification of carbon nanotubes with stable thermoelectric performance at high temperature [J ] . Chemical Engineering Journal , 2025 , 506 : 160213 .

XIE W H , YAO X Y , LI H , et al . Biomass-based N-rich porous carbon materials for CO 2 capture and in-situ conversion [J ] . ChemSusChem , 2022 , 15 ( 18 ): e202201004 .

LI H N , YANG H C , ZHU C Y , et al . A self-descaling Janus nanofibrous evaporator enabled by a “moving interface” for durable solar-driven desalination of hypersaline water [J ] . Journal of Materials Chemistry A , 2022 , 10 ( 39 ): 20856 - 20865 .

LI X , ZHANG K , NILGHAZ A , et al . A green and sustainable water evaporation-induced electricity generator with woody biochar [J ] . Nano Energy , 2023 , 112 : 108491 .

BAI W C , YANG X C , SONG X W , et al . Advanced solar-driven hydrogel sponge for efficient heavy metal wastewater purification and clean water production through interfacial evaporation [J ] . Environmental Research , 2025 , 264 : 120322 .

TAO P , NI G , SONG C Y , et al . Solar-driven interfacial evaporation [J ] . Nature Energy , 2018 , 3 ( 12 ): 1031 - 1041 .

WEN J , LI X K , ZHANG H , et al . Architecting Janus hydrogel evaporator with polydopamine-TiO 2 photocatalyst for high-efficient solar desalination and purification [J ] . Separation and Purification Technology , 2023 , 304 : 122403 .

CHANG M M , YANG R R , LAI X J , et al . Photothermic-catalytic bifunctionality of boron-doped molybdenum disulfide nanosheets enabling simultaneous solar evaporation and antibiotic destruction [J ] . Chemical Engineering Journal , 2024 , 499 : 156716 .

WANG S W , WANG F Z , LV B W , et al . Three-Dimensional evaporator for simultaneous VOC removal and clean water production [J ] . Separation and Purification Technology , 2024 , 351 : 128051 .

LI X K , YANG R , ZOU L , et al . Reassessing the role of thermal convection in simultaneous water production and pollutant degradation in interfacial photothermal-photocatalytic systems [J ] . Advanced Materials , 2025 , 37 ( 4 ): 2416283 .

ZHAO D M , DING M C , LIN T H , et al . Gradient graphene spiral sponges for efficient solar evaporation and zero liquid discharge desalination with directional salt crystallization [J ] . Advanced Science , 2024 , 11 ( 22 ): 2400310 .

ZOU H , YANG X G , ZHU J L , et al . Solar-driven scalable hygroscopic gel for recycling water from passive plant transpiration and soil evaporation [J ] . Nature Water , 2024 , 2 ( 7 ): 663 - 673 .

YAO J R , ZHONG Q Y , ZHANG J , et al . Interfacial solar evaporation for zero liquid discharge desalination [J ] . Communications Materials , 2024 , 5 ( 1 ): 103 .

ZHONG L B , CHEN S J , HOU X , et al . Salt-resistant carbon aerogel with hierarchical interconnected channels for continuous and efficient solar evaporation of hypersaline water [J ] . Science China Materials , 2023 , 66 ( 8 ): 3300 - 3309 .

CHANG C , TAO P , XU J L , et al . High-efficiency superheated steam generation for portable sterilization under ambient pressure and low solar flux [J ] . ACS Applied Materials & Interfaces , 2019 , 11 ( 20 ): 18466 - 18474 .

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