粉煤灰源硅基固体胺吸附剂捕集CO<sub>2</sub>的研究进展

廖清云; 杨茜; 赵潇; 栗晟; 王骥; 刘涛

doi:10.12434/j.issn.2097-2547.20240275

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粉煤灰源硅基固体胺吸附剂捕集CO₂的研究进展

CCUS技术 | 更新时间：2025-03-27

- 粉煤灰源硅基固体胺吸附剂捕集CO₂的研究进展
- Research progress of silicon-based solid amine adsorbents derived from fly ash for CO₂ capture
- 低碳化学与化工 2025, 50(3): 106-112.
- 作者机构：
  
  1.天府永兴实验室 CO2捕集新原理与技术研究中心，四川成都 610213
  2.四川大学新能源与低碳技术研究院，四川成都 610065
- 作者简介：
  
  廖清云（1996—），博士，助理研究员，研究方向为CO2捕集与利用，E-mail：qingyun9196@foxmail.com。
  刘涛（1990—），博士，研究员，研究方向为CO2捕集与利用和零碳氢能制备，E-mail：liutao3200023@scu.edu.cn。
- 基金信息：
  
  天府永兴实验室有组织科研项目(2023CXXM24;2023KJGG02;2023KJGG01)
- DOI：10.12434/j.issn.2097-2547.20240275
  中图分类号： TQ424
- 收稿日期：2024-06-25，
  
  修回日期：2024-07-21，
  
  纸质出版日期：2025-03-25
- 稿件说明：
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廖清云,杨茜,赵潇等.粉煤灰源硅基固体胺吸附剂捕集CO₂的研究进展[J].低碳化学与化工,2025,50(03):106-112.

LIAO Qingyun,YANG Qian,ZHAO Xiao,et al.Research progress of silicon-based solid amine adsorbents derived from fly ash for CO₂ capture[J].Low-carbon Chemistry and Chemical Engineering,2025,50(03):106-112.
廖清云,杨茜,赵潇等.粉煤灰源硅基固体胺吸附剂捕集CO₂的研究进展[J].低碳化学与化工,2025,50(03):106-112. DOI： 10.12434/j.issn.2097-2547.20240275.

LIAO Qingyun,YANG Qian,ZHAO Xiao,et al.Research progress of silicon-based solid amine adsorbents derived from fly ash for CO₂ capture[J].Low-carbon Chemistry and Chemical Engineering,2025,50(03):106-112. DOI： 10.12434/j.issn.2097-2547.20240275.

摘要

纳米二氧化硅高昂的合成成本制约了硅基固体胺吸附剂的进一步推广应用。固废资源粉煤灰中二氧化硅含量较高，以粉煤灰为硅源降低硅基固体胺吸附剂制备成本逐渐成为研究热点。综述了近年来粉煤灰源硅基固体胺吸附剂的研究进展，重点阐述了粉煤灰源

硅基固体胺吸附剂的基体制备技术、有机胺负载技术、CO

吸附性能和循环稳定性，并对现有粉煤灰源硅基固体胺吸附剂存在的问题进行了分析。最后对粉煤灰源硅基固体胺吸附剂未来研究方向进行了展望。

Abstract

The high synthetic cost of nano-silicon restricts the further application of silicon-based solid amine adsorbents. The content of silicon in fly ash is high

so using fly ash as silicon source to reduce the preparation cost of silicon-based solid amine adsorbent has become a research focus. The research progress of silicon-based solid amine adsorbents derived from fly ash in recent years was reviewed. And the substrate preparation technologies

organic amine loading technologies

adsorption performances and cycle stabilities of silicon-based solid amine adsorbents derived from fly ash were emphatically described. Finally

the future research directions of silicon-based solid amine adsorbents derived from fly ash were prospected.

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references

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粉煤灰源硅基固体胺吸附剂捕集CO2的研究进展

Research progress of silicon-based solid amine adsorbents derived from fly ash for CO2 capture

DOI：10.12434/j.issn.2097-2547.20240275

摘要

Abstract

关键词

Keywords

references

粉煤灰源硅基固体胺吸附剂捕集CO₂的研究进展

Research progress of silicon-based solid amine adsorbents derived from fly ash for CO₂ capture