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Effects of SO2, H2O and O2 in coal-fired flue gas on solid CO2 adsorbents: Mechanisms and modification strategies
| 更新时间：2026-04-17
|
Effects of SO2, H2O and O2 in coal-fired flue gas on solid CO2 adsorbents: Mechanisms and modification strategies
- Low-Carbon Chemistry and Chemical Engineering Pages: 1-15(2026)
- 作者机构：
1.太原理工大学 省部共建煤基能源清洁高效利用国家重点实验室，山西 太原 030024
2.太原理工大学 化学与化工学院，山西 太原 030024
- 作者简介：
- 基金信息：
DOI：10.12434/j.issn.2097-2547.20250479
CLC： TQ424Received：18 December 2025，
Revised：2025-12-25，
Online First：15 April 2026，
- 稿件说明：
移动端阅览
刘雨欣,徐玉凤,荆洁颖.燃煤烟气中SO2、H2O和O2对固体CO2吸附剂的影响机制与改性策略[J].低碳化学与化工,
LIU Yuxin,XU Yufeng,JING Jieying.Effects of SO2, H2O and O2 in coal-fired flue gas on solid CO2 adsorbents: Mechanisms and modification strategies[J].Low-Carbon Chemistry and Chemical Engineering,
刘雨欣,徐玉凤,荆洁颖.燃煤烟气中SO2、H2O和O2对固体CO2吸附剂的影响机制与改性策略[J].低碳化学与化工, DOI：10.12434/j.issn.2097-2547.20250479.
LIU Yuxin,XU Yufeng,JING Jieying.Effects of SO2, H2O and O2 in coal-fired flue gas on solid CO2 adsorbents: Mechanisms and modification strategies[J].Low-Carbon Chemistry and Chemical Engineering, DOI：10.12434/j.issn.2097-2547.20250479.
Effects of SO2, H2O and O2 in coal-fired flue gas on solid CO2 adsorbents: Mechanisms and modification strategies
摘要
燃煤烟气CO
2
捕集是实现碳减排的关键环节，高效稳定的固体CO
2
吸附剂是该环节的核心。然而，实际烟气中的杂质气体（如H
2
O、O
2
和SO
2
）会劣化吸附剂结构并降低其CO
2
吸附性能，这对CO
2
捕集技术的应用产生了不利影响。阐述了SO
2
、H
2
O和O
2
对典型固体CO
2
吸附剂（如CaO基、MgO基和固体胺吸附剂）吸附性能的影响，并总结了针对性改性策略。目前研究多关注单一杂质的影响，同时改性方法存在成本过高和工艺复杂等问题。未来研究可考虑多种杂质共存的影响，并优化吸附剂改性策略，以期开发兼具高吸附性能和高稳定性，并能适应复杂条件的CO
2
吸附剂。
Abstract
CO
2
capture from coal-fired flue gas is a critical step in achieving carbon emissions reduction
and highly efficient and stable solid CO
2
adsorbents are central to this process. However
impurity gas
es (such as H
2
O
O
2
and SO
2
) in actual flue gas can degrade the adsorbent structure and reduce its CO
2
adsorption performance
which adversely affects the application of CO
2
capture technologies. Effects of SO
2
H
2
O and O
2
on adsorption performance of typical solid CO
2
adsorbents (such as CaO-based
MgO-based and solid amine adsorbents) were described and targeted modification strategies were summarized. Current research often focuses on the effect of a single impurity
while existing modification methods suffer from issues such as high costs and complex processes. Future research can consider the effects of multiple coexisting impurities and optimize adsorbent modification strategies to develop CO
2
adsorbents that combine high adsorption performances and stabilities while being capable of operating under complex conditions.
关键词
Keywords
references
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School of Resources and Safety Engineering, Chongqing University
National Institute of Metrology
National Energy Group New Energy Technology Research Institute Co., Ltd.
College of Chemical and Pharmaceutical Engineering, Wuhan Institute of Technology
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